Her first movie role was as Molly in Heart of the Beholder (2005), a story about a family who opened the first video cassette store in 1980. This was followed by a small role in Family Plan (2005) (TV) as Young Charlie.She appeared in her first big film: the remake of the classic film,The Amityville Horror.At the time of the film's release,Chloë was so young that she was not allowed to see it with the rest of the cast at the film's premiere.Chloë biggest break came in 2010, when she took on the controversial role of Mindy Macready, aka Hit-Girl, in Matthew Vaughn's film adaptation of Mark Millar's popular graphic novel series, Kick-Ass.Thanks to her intense training for the film, Chloë is trained in martial arts and weapons handling.
Chloë's approach to acting has been consisten: "I always try to find something in my own life that connects me to the character. The more I live, the more I find things that I can use in my acting." She adds, "I have learned never to judge any of the characters that I protray. Sometimes that is difficult to di, because as a human being, we tend to make judgments when we find out information about people and situations.
To date, Chloë has been involved in over 20 film productions, guest starred in numerous television show (includin a two-yeas stint on Disney's "My Friends Tigger & Pooh"), and has appeared in music video for best Coast and the Soft Pack.